You dont need a lot of force to hold the mold together, what is important is that the force is distributed evenly and flat.
you always want the rubber bands to be as close to the mold as posslble, even going over the top of the molds as well if they do not get in the way of the pour.
THe sprue design is very wastefull of resin and rubber!
see attached image I made-
On the left- optimum design for a single peice split mold, blue line indicted the depth of the split. for this style you would pour, squeeze, pour squeeze untill no more bubbles come out, then pressureise it, also hammer it on the table abit while you squeeze.
on the right- optimum design for a two part mold- pour into the fill channel while hammering your fist next to the mold, untill you see resin in the air vents, no sqeezing required for this style, just pressure ideally.
To help with mold alignment and make the mold quickier, you could actually pour it as a single pour if you designed hte sprue correctly, then cut it like a split mold almost to the bottom, so the two "halves" are actually still attached. the blue line on the right mold shows whre this cut line would go.
hope ths helps,
AH